000145651 001__ 145651
000145651 005__ 20250923084438.0
000145651 0247_ $$2doi$$a10.1039/d4nr03484h
000145651 0248_ $$2sideral$$a140522
000145651 037__ $$aART-2024-140522
000145651 041__ $$aeng
000145651 100__ $$aRepollés, Ana
000145651 245__ $$aAsymmetric [Dy2] molecules deposited into microSQUID susceptometers: in situ characterization of their magnetic integrity
000145651 260__ $$c2024
000145651 5060_ $$aAccess copy available to the general public$$fUnrestricted
000145651 5203_ $$aThe controlled integration of magnetic molecules into superconducting circuits is key to developing hybrid quantum devices. Herein, we study [Dy2] molecular dimers deposited into micro-SQUID susceptometers. The results of magnetic, heat capacity and magnetic resonance experiments, backed by theoretical calculations, show that each [Dy2] dimer fulfills the main requisites to encode a two-spin quantum processor. Arrays of between 2 * 108 and 7 * 109[Dy2] molecules were optimally integrated under ambient conditions inside the 20 mum wide loops of micro-SQUID sensors by means of dip-pen nanolithography. Equilibrium magnetic susceptibility and phonon-assisted spin tunneling dynamics measured in situ substantiate that these molecules preserve spin ground states, magnetic interactions and magnetic asymmetry that characterize them in bulk. These results show that it is possible to interface multi-qubit molecular complexes with on-chip superconducting circuits without disturbing their relevant properties and suggest the potential of soft nanolithography techniques to achieve this goal.
000145651 536__ $$9info:eu-repo/grantAgreement/ES/AEI/AEI PID2022-140923NB-C21$$9info:eu-repo/grantAgreement/ES/DGA/E09-23R$$9info:eu-repo/grantAgreement/ES/DGA/E31-23R$$9info:eu-repo/grantAgreement/ES/MICINN-AEI/PRTR-C17.I1$$9info:eu-repo/grantAgreement/ES/MICINN/PDC2022-133184-I00$$9info:eu-repo/grantAgreement/ES/MICINN/PID2020-1183294RB-I00$$9info:eu-repo/grantAgreement/ES/MICINN/PID2022-137764OB-I00$$9info:eu-repo/grantAgreement/EUR/MICINN/TED2021-129214B-I00$$9info:eu-repo/grantAgreement/EUR/MICINN/TED2021-131447B-C21
000145651 540__ $$9info:eu-repo/semantics/openAccess$$aby-nc$$uhttp://creativecommons.org/licenses/by-nc/3.0/es/
000145651 590__ $$a5.1$$b2024
000145651 592__ $$a1.245$$b2024
000145651 591__ $$aPHYSICS, APPLIED$$b45 / 187 = 0.241$$c2024$$dQ1$$eT1
000145651 593__ $$aNanoscience and Nanotechnology$$c2024$$dQ1
000145651 591__ $$aNANOSCIENCE & NANOTECHNOLOGY$$b53 / 147 = 0.361$$c2024$$dQ2$$eT2
000145651 593__ $$aMaterials Science (miscellaneous)$$c2024$$dQ1
000145651 591__ $$aCHEMISTRY, MULTIDISCIPLINARY$$b67 / 239 = 0.28$$c2024$$dQ2$$eT1
000145651 591__ $$aMATERIALS SCIENCE, MULTIDISCIPLINARY$$b141 / 460 = 0.307$$c2024$$dQ2$$eT1
000145651 655_4 $$ainfo:eu-repo/semantics/article$$vinfo:eu-repo/semantics/publishedVersion
000145651 700__ $$aPallarés, María Carmen
000145651 700__ $$aAguilà, David
000145651 700__ $$aRoubeau, Olivier
000145651 700__ $$aVelasco, Verónica
000145651 700__ $$aGella, Diego
000145651 700__ $$aBarrios, Leoní A.
000145651 700__ $$0(orcid)0000-0002-8125-877X$$aMartínez-Pérez, María José
000145651 700__ $$0(orcid)0000-0002-7742-9329$$aSesé, Javier
000145651 700__ $$aDrung, Dietmar
000145651 700__ $$0(orcid)0000-0002-5406-3280$$aMartínez, Jesús Ignacio$$uUniversidad de Zaragoza
000145651 700__ $$aSchurig, Thomas
000145651 700__ $$aLe Guennic, Boris
000145651 700__ $$0(orcid)0000-0001-7460-5916$$aLostao, Anabel
000145651 700__ $$aAromí, Guillem
000145651 700__ $$0(orcid)0000-0001-6284-0521$$aLuis, Fernando
000145651 7102_ $$12003$$2395$$aUniversidad de Zaragoza$$bDpto. Física Materia Condensa.$$cÁrea Física Materia Condensada
000145651 773__ $$g17, 1 (2024), 219-229$$pNanoscale$$tNanoscale$$x2040-3364
000145651 8564_ $$s5478232$$uhttps://zaguan.unizar.es/record/145651/files/texto_completo.pdf$$yVersión publicada
000145651 8564_ $$s2838040$$uhttps://zaguan.unizar.es/record/145651/files/texto_completo.jpg?subformat=icon$$xicon$$yVersión publicada
000145651 909CO $$ooai:zaguan.unizar.es:145651$$particulos$$pdriver
000145651 951__ $$a2025-09-22-14:48:35
000145651 980__ $$aARTICLE