000061000 001__ 61000 000061000 005__ 20200221144325.0 000061000 0247_ $$2doi$$a10.1080/00102202.2016.1138824 000061000 0248_ $$2sideral$$a93366 000061000 037__ $$aART-2016-93366 000061000 041__ $$aeng 000061000 100__ $$0(orcid)0000-0001-7559-9669$$aAbián, M. 000061000 245__ $$aInteraction soot-SO2. Experimental and kinetic analysis 000061000 260__ $$c2016 000061000 5060_ $$aAccess copy available to the general public$$fUnrestricted 000061000 5203_ $$aThis study aims to evaluate the capability of SO2 to interact with soot and to determine the kinetics of this reaction under conditions of interest for combustion. The conditions of the soot reactivity experiments were: 1% SO2 with nitrogen to balance, around 10 mg of soot, and different reaction temperatures for each run: 1275, 1325, 1375, 1425, and 1475 K. Results demonstrate that SO2 does interact with soot. The evaluation of the soot reactivity has been based on the calculation of the time for the complete conversion of carbon through the employment of the Shrinking Core Model equations for decreasing size particle with chemical reaction control. The reactivity of soot with SO2 increased by a factor of about 3 when increasing the reaction temperature of the test from 1275 K to 1475 K. Kinetics in terms of Arrhenius parameters showed that the activation energy of the interaction of soot with SO2 was around 82 kJ/mol. 000061000 536__ $$9info:eu-repo/grantAgreement/ES/MINECO/CTQ2012-34423$$9info:eu-repo/grantAgreement/ES/MINECO/FPDI-2013-16172 000061000 540__ $$9info:eu-repo/semantics/openAccess$$aby$$uhttp://creativecommons.org/licenses/by/3.0/es/ 000061000 590__ $$a1.241$$b2016 000061000 591__ $$aENGINEERING, MULTIDISCIPLINARY$$b36 / 85 = 0.424$$c2016$$dQ2$$eT2 000061000 591__ $$aTHERMODYNAMICS$$b35 / 58 = 0.603$$c2016$$dQ3$$eT2 000061000 591__ $$aENERGY & FUELS$$b63 / 92 = 0.685$$c2016$$dQ3$$eT3 000061000 591__ $$aENGINEERING, CHEMICAL$$b82 / 135 = 0.607$$c2016$$dQ3$$eT2 000061000 592__ $$a0.416$$b2016 000061000 593__ $$aChemical Engineering (miscellaneous)$$c2016$$dQ2 000061000 593__ $$aChemistry (miscellaneous)$$c2016$$dQ2 000061000 593__ $$aPhysics and Astronomy (miscellaneous)$$c2016$$dQ2 000061000 593__ $$aFuel Technology$$c2016$$dQ2 000061000 593__ $$aEnergy Engineering and Power Technology$$c2016$$dQ2 000061000 655_4 $$ainfo:eu-repo/semantics/article$$vinfo:eu-repo/semantics/acceptedVersion 000061000 700__ $$0(orcid)0000-0001-5426-6486$$aMillera, A.$$uUniversidad de Zaragoza 000061000 700__ $$0(orcid)0000-0002-5420-0943$$aBilbao, R.$$uUniversidad de Zaragoza 000061000 700__ $$0(orcid)0000-0003-4679-5761$$aAlzueta, M.U.$$uUniversidad de Zaragoza 000061000 7102_ $$15005$$2555$$aUniversidad de Zaragoza$$bDpto. Ing.Quím.Tecnol.Med.Amb.$$cÁrea Ingeniería Química 000061000 7102_ $$15005$$2790$$aUniversidad de Zaragoza$$bDpto. Ing.Quím.Tecnol.Med.Amb.$$cÁrea Tecnologi. Medio Ambiente 000061000 773__ $$g188, 4-5 (2016), 482-491$$pCombust. sci. technol.$$tCOMBUSTION SCIENCE AND TECHNOLOGY$$x0010-2202 000061000 8564_ $$s911834$$uhttps://zaguan.unizar.es/record/61000/files/texto_completo.pdf$$yPostprint 000061000 8564_ $$s26021$$uhttps://zaguan.unizar.es/record/61000/files/texto_completo.jpg?subformat=icon$$xicon$$yPostprint 000061000 909CO $$ooai:zaguan.unizar.es:61000$$particulos$$pdriver 000061000 951__ $$a2020-02-21-13:43:27 000061000 980__ $$aARTICLE