000089985 001__ 89985
000089985 005__ 20210902121825.0
000089985 0247_ $$2doi$$a10.1002/anie.202005558
000089985 0248_ $$2sideral$$a118366
000089985 037__ $$aART-2020-118366
000089985 041__ $$aeng
000089985 100__ $$aWatts, A.
000089985 245__ $$aSite-Specific Iron Substitution in STA-28, a Large Pore Aluminophosphate Zeotype Prepared Using 1, 10-Phenanthrolines as Framework-Bound Templates
000089985 260__ $$c2020
000089985 5060_ $$aAccess copy available to the general public$$fUnrestricted
000089985 5203_ $$aAn AlPO 4 zeotype has been prepared using the aromatic diamine 1,10‐phenanthroline and some of its methylated analogues as templates. In each case the two template N atoms bind to a specific framework Al site to expand its coordination to the unusual octahedral AlO 4 N 2 environment. Furthermore, using this framework‐bound template, Fe atoms can be included selectively at this site in the framework by direct synthesis, as confirmed by annular dark field scanning transmission electron microscopy and Rietveld refinement. Calcination removes the organic molecules to give large pore framework solids, with BET surface areas up to 540 m 2 g ‐1 and two perpendicular sets of channels that intersect to give pore space connected by 12‐ring openings along all crystallographic directions.
000089985 536__ $$9info:eu-repo/grantAgreement/ES/MICINN/RYC-2018-024561-I
000089985 540__ $$9info:eu-repo/semantics/openAccess$$aby$$uhttp://creativecommons.org/licenses/by/3.0/es/
000089985 590__ $$a15.336$$b2020
000089985 591__ $$aCHEMISTRY, MULTIDISCIPLINARY$$b16 / 178 = 0.09$$c2020$$dQ1$$eT1
000089985 592__ $$a5.831$$b2020
000089985 593__ $$aChemistry (miscellaneous)$$c2020$$dQ1
000089985 593__ $$aCatalysis$$c2020$$dQ1
000089985 655_4 $$ainfo:eu-repo/semantics/conferenceObject$$vinfo:eu-repo/semantics/publishedVersion
000089985 700__ $$aLozinska, M.
000089985 700__ $$aSlawin, A.
000089985 700__ $$0(orcid)0000-0002-5229-2717$$aMayoral, A.$$uUniversidad de Zaragoza
000089985 700__ $$aDawson, D.
000089985 700__ $$aAshbrook, S.
000089985 700__ $$aBode, B.
000089985 700__ $$aDugulan, I.
000089985 700__ $$aShannon, M.
000089985 700__ $$aCox, P.
000089985 700__ $$aTurrina, A.
000089985 700__ $$aWright, P. A.
000089985 7102_ $$12003$$2395$$aUniversidad de Zaragoza$$bDpto. Física Materia Condensa.$$cÁrea Física Materia Condensada
000089985 773__ $$g59, 35 (2020), 15186 - 15190$$pAngew. Chem. (Int. ed.)$$tAngewandte Chemie - International Edition$$x1433-7851
000089985 8564_ $$s1540107$$uhttps://zaguan.unizar.es/record/89985/files/texto_completo.pdf$$yVersión publicada
000089985 8564_ $$s34167$$uhttps://zaguan.unizar.es/record/89985/files/texto_completo.jpg?subformat=icon$$xicon$$yVersión publicada
000089985 909CO $$ooai:zaguan.unizar.es:89985$$particulos$$pdriver
000089985 951__ $$a2021-09-02-10:11:09
000089985 980__ $$aARTICLE