000096085 001__ 96085
000096085 005__ 20210507081953.0
000096085 0247_ $$2doi$$a10.1039/c9cy02128k
000096085 0248_ $$2sideral$$a114681
000096085 037__ $$aART-2019-114681
000096085 041__ $$aeng
000096085 100__ $$aSorribes, Iván
000096085 245__ $$aPalladium doping of In2O3 towards a general and selective catalytic hydrogenation of amides to amines and alcohols
000096085 260__ $$c2019
000096085 5060_ $$aAccess copy available to the general public$$fUnrestricted
000096085 5203_ $$aHerein, the first general heterogeneous catalytic protocol for the hydrogenation of primary, secondary and tertiary amides to their corresponding amines and alcohols is described. Advantageously, this catalytic protocol works under additive-free conditions and is compatible with the presence of aromatic rings, which are fully retained in the final products. This hydrogenative C-N bond cleavage methodology is catalyzed by a Pd-doped In2O3 catalyst prepared by a microwave hydrothermal-assisted method followed by calcination. This catalyst displays highly dispersed Pd2+ ionic species in the oxide matrix of In2O3 that have appeared to be essential for its high catalytic performance.
000096085 536__ $$9info:eu-repo/grantAgreement/ES/DGA-FEDER/Construyendo Europa desde Aragón$$9info:eu-repo/grantAgreement/ES/DGA-FEDER/E31-17R$$9info:eu-repo/grantAgreement/ES/MICINN/Juan de la Cierva Program-IJCI-2016-30590$$9info:eu-repo/grantAgreement/ES/MINECO-FEDER/PGC2018-094417-B-I00
000096085 540__ $$9info:eu-repo/semantics/openAccess$$aAll rights reserved$$uhttp://www.europeana.eu/rights/rr-f/
000096085 590__ $$a5.721$$b2019
000096085 591__ $$aCHEMISTRY, PHYSICAL$$b41 / 159 = 0.258$$c2019$$dQ2$$eT1
000096085 592__ $$a1.579$$b2019
000096085 593__ $$aCatalysis$$c2019$$dQ1
000096085 655_4 $$ainfo:eu-repo/semantics/article$$vinfo:eu-repo/semantics/acceptedVersion
000096085 700__ $$aLemos, Samantha CS
000096085 700__ $$0(orcid)0000-0001-9193-3874$$aMartín, Santiago$$uUniversidad de Zaragoza
000096085 700__ $$0(orcid)0000-0002-5229-2717$$aMayoral, Álvaro
000096085 700__ $$aLima, Renata C
000096085 700__ $$aAndres, Juan
000096085 7102_ $$12012$$2755$$aUniversidad de Zaragoza$$bDpto. Química Física$$cÁrea Química Física
000096085 773__ $$g9, 24 (2019), 6965-6976$$pCATALYSIS SCIENCE & TECHNOLOGY$$tCatalysis Science and Technology$$x2044-4753
000096085 8564_ $$s1193602$$uhttps://zaguan.unizar.es/record/96085/files/texto_completo.pdf$$yPostprint
000096085 8564_ $$s545325$$uhttps://zaguan.unizar.es/record/96085/files/texto_completo.jpg?subformat=icon$$xicon$$yPostprint
000096085 909CO $$ooai:zaguan.unizar.es:96085$$particulos$$pdriver
000096085 951__ $$a2021-05-07-08:11:52
000096085 980__ $$aARTICLE