Suppression of ferromagnetism and emergence of spin-glass-like behavior in the CuCr2-x Snx S2 Se2 spinels
Resumen: Magnetometry, neutron diffraction experiments, and high-resolution transmission electron microscopy (HRTEM) were performed to study the magnetic behavior of CuCr2−⁢Sn⁢S2⁢Se2 (0.2≤≤1.0) solid solutions and experimentally determine the appropriate magnetic structure for these systems. For all samples, the main phase with normal spinel-type structure (⁢⁢ 3 ⁢) was refined. For low Sn concentration a minority monoclinic phase appears also corroborated with HRTEM analyses. Together with the results from magnetization experiments, neutron diffraction measurements allowed to establish that for samples with ≤0.4 there is a ferromagnetic long-range order at high temperatures labeled with the 3⁢ irrep m⁢Γ+ 4 of ⁢⁢ ‾ 3 ⁢.1′, while for >0.4 no magnetic signal is observed, indicating that the ferromagnetic behavior is suppressed and replaced with a spin-glass-like state.
Idioma: Inglés
DOI: 10.1103/PhysRevB.110.064436
Año: 2024
Publicado en: Physical Review B 110, 6 (2024)
ISSN: 2469-9950

Factor impacto JCR: 3.7 (2024)
Categ. JCR: MATERIALS SCIENCE, MULTIDISCIPLINARY rank: 208 / 461 = 0.451 (2024) - Q2 - T2
Categ. JCR: PHYSICS, CONDENSED MATTER rank: 30 / 80 = 0.375 (2024) - Q2 - T2
Categ. JCR: PHYSICS, APPLIED rank: 66 / 187 = 0.353 (2024) - Q2 - T2

Factor impacto CITESCORE: 6.2 - Condensed Matter Physics (Q1) - Electronic, Optical and Magnetic Materials (Q2)

Factor impacto SCIMAGO: 1.303 - Electronic, Optical and Magnetic Materials (Q1) - Condensed Matter Physics (Q1)

Tipo y forma: Article (PostPrint)

Creative Commons You must give appropriate credit, provide a link to the license, and indicate if changes were made. You may do so in any reasonable manner, but not in any way that suggests the licensor endorses you or your use. You may not use the material for commercial purposes. If you remix, transform, or build upon the material, you may not distribute the modified material.


Exportado de SIDERAL (2026-02-17-20:38:15)


Visitas y descargas

Este artículo se encuentra en las siguientes colecciones:
Articles



 Record created 2024-10-03, last modified 2026-02-17


Postprint:
 PDF
Rate this document:

Rate this document:
1
2
3
 
(Not yet reviewed)